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You should be able to do that. You'd create a "Sandbox - shared users" on the SSD. That'll copy everything but the contents of /Users to the SSD.
Time Machine will likely recopy everything from both drives if you do this..but I believe it will run normally after. Note that you'll want to back up the main drive, for the most part - you'd going to use this just like a regular Sandbox.
Hope that helps!
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--Dave Nanian
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